Columbia's parent company Sony Music Entertainment released ten of the band's Columbia songs in a Super Hits compilation in May 1994, which was certified gold in 2002. Shenandoah also collaborated with country and bluegrass singer Ricky Skaggs on the 1994 Keith Whitley tribute Keith Whitley: A Tribute Album, recording a cover version of Whitley's "All I Ever Loved Was You". Later in 1994, the band left RCA for Liberty Records, then the name for the Nashville division of Capitol Records. RCA gave Liberty the master recordings for a nearly-completed album, to which Liberty added "Somewhere in the Vicinity of the Heart", a song featuring guest vocals from bluegrass musician Alison Krauss. Liberty released the album in November 1994 as In the Vicinity of the Heart, with the number seven-peaking title track also serving as the first single release. This song was also Krauss' first top 40 country hit, and its success helped boost sales of her album Now That I've Found You: A Collection.  Vicinity became the band's fastest-selling album, and the first 175,000 copies were distributed with prepaid telephone cards which included an 800 number that could be called to receive a greeting from the band members. The album also produced the band's last Top Ten hit in "Darned If I Don't (Danged If I Do)." Originally the B-side to "Somewhere in the Vicinity of the Heart," this song was co-written by Ronnie Dunn (of Brooks & Dunn) and songwriter Dean Dillon, best known for co-writing several of George Strait's singles. "Heaven Bound (I'm Ready)" (another Dennis Linde song) and "Always Have, Always Will," peaking at numbers 24 and 40, were the last two releases from the album. Jim Ridley gave the album a two-and-a-half star rating in New Country magazine, citing the vocal performances on the title track and "I Wouldn't Know" as standouts, but saying that the rest of the album did not take any risks.  Raybon released a solo gospel music album for Sparrow Records in July 1995, and in October of the same year, that label released a multi-artist country-gospel album entitled Amazing Grace -- A Country Salute to Gospel, to which the band contributed a rendition of "Beulah Land." Shenandoah also covered The Beatles' "Can't Buy Me Love" on the mid-1995 album Come Together: America Salutes The Beatles. "Somewhere in the Vicinity of the Heart" won Shenandoah and Krauss won the 1995 Grammy Award for Best Country Vocal Collaboration and the Country Music Association award for Vocal Event, and "Darned If I Don't" was nominated for Grammy Award for Best Country Vocal by a Duo or Group the same year.

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a nearly-completed album, to which Liberty added "Somewhere in the Vicinity of the Heart", a song featuring guest vocals from bluegrass musician Alison Krauss.