Li Lykke Timotej Zachrisson was born in Ystad, Skane; her mother, Karsti Stiege, was a photographer, and her father, Johan Zachrisson (stage name Zilverzurfarn), is a member of the Swedish punk-reggae band Dag Vag. The family moved to Stockholm when Zachrisson was a toddler and when she was six moved to a mountaintop in Portugal where they lived for five years. The family also spent time in Lisbon and Morocco, and winters in Nepal and India. She moved to the neighborhood of Bushwick in Brooklyn, New York City, for three months when she was 19.

The song "Get Some" was featured in the 15th episode of the first season of Hawaii Five-0 titled "Kai e'e" which aired 23 January 2011. The song was also used in ABC Family's drama Pretty Little Liars in the 18th episode of the second season which was titled "A Kiss Before Lying" which aired 30 January 2012. The song was also used in the 19th episode of the second season of The CW's The Vampire Diaries, titled "Klaus" and originally aired 21 April 2011, as well as the sixth episode of the first season of Teen Wolf, titled "Heart Monitor" and originally aired 4 July 2011. The song was also used in the film Premium Rush as one of its soundtracks. The song "Unrequited Love" was used in episode 19 ("The Wheels of Justice"), season four of The Good Wife.  Li's song "Melodies and Desires" was featured in the 2010 Australian film Griff the Invisible and an edited version of "Get Some" was featured in the Catwoman trailer for the video game, Batman: Arkham City. She collaborated with singer Kleerup on the song "Until We Bleed", which was featured on an episode of UK TV series Misfits and an episode of the television series Ringer.  Her second album Wounded Rhymes was released in 2011. The album was featured on several lists of 2011's best albums, including Q, Mojo, The Observer, The New York Times, The Huffington Post and Rolling Stone. The 19 April 2011, episode of Glee (titled "A Night of Neglect") featured student Tina singing a version of Li's "I Follow Rivers". On 30 April 2011, she performed on Later... with Jools Holland in the UK, playing "Get Some", "Sadness Is a Blessing" and "I Follow Rivers". Li played at the 2011 Latitude Festival, held between 14 and 18 July 2011 at Henham Park in Suffolk, England. She appeared with her band on US late night talk show The Tonight Show with Jay Leno in August 2011 and on the Late Show with David Letterman in November 2011.  Belgian DJ/producer The Magician's remix of "I Follow Rivers" is featured in Jacques Audiard's 2012 film Rust and Bone and the 2013 Palme d'Or-winning Blue Is the Warmest Colour. Li contributed to the 2012 compilation "Volym 1" with the track "Come Near" released by the Swedish artist collective and record label INGRID where she is a founding member. She also contributed a cover of "Silver Springs" to a 2012 Fleetwood Mac tribute album, which included renditions from Best Coast, Marianne Faithfull, and MGMT.  In 2013, she was featured as a guest musician on David Lynch's second studio album The Big Dream, performing vocals on the lead single "I'm Waiting Here".

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